Print Email Facebook Twitter Predicting Aerosol Based Emissions in a Post Combustion CO2 Capture Process Using an Aspen Plus Model Title Predicting Aerosol Based Emissions in a Post Combustion CO2 Capture Process Using an Aspen Plus Model Author Khakharia, P.M. Mertens, J. Vlugt, T.J.H. Goetheer, E. Faculty Mechanical, Maritime and Materials Engineering Department Process and Energy Date 2014-10-05 Abstract Industrial scale implementation of post combustion CO2 capture (PCCC) can be hindered by solvent emissions due to its impact on the environment and the operating costs. The issue of aerosol based emissions has only been recently reported for a PCCC process and very little fundamental knowledge is available in the scientific community on this topic. Therefore, it is important to understand the mechanism of aerosol formation and growth so that appropriate countermeasures can be applied in reducing the total emissions. In this study, a simplified methodology is presented for predicting aerosol based emissions from a CO2 capture column of a PCCC process. The basis of this methodology is to split the counter-current gas-liquid interaction from the cocurrent gas-aerosol interaction. The absorption column is discretised into multiple alternating gas-liquid and gas-aerosol sections in Aspen Plus with an assumption that aerosols behave as a continuous phase rather droplets. The degree of supersaturation, which is important for aerosol formation and growth, is calculated along the column. The effect of the changes in parameters of the PCCC plant, such as the CO2 content of the inlet flue gas, the lean solvent temperature and the lean solvent loading on aerosol based emissions are investigated. The aerosol based emissions follows the trend of the supersaturation ratio in the absorber column. To reference this document use: http://resolver.tudelft.nl/uuid:7f884a5f-afdd-4115-b60f-9cd9885dae3e Publisher Elsevier ISSN 1876-6102 Source https://doi.org/10.1016/j.egypro.2014.11.101 Source Energy Procedia, 63, 2014; 12th International Conference on Greenhouse Gas Control Technologies, GHGT-12 Part of collection Institutional Repository Document type journal article Rights © 2014 This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/3.0/) Files PDF 318942.pdf 582.33 KB Close viewer /islandora/object/uuid:7f884a5f-afdd-4115-b60f-9cd9885dae3e/datastream/OBJ/view